埃達克岩與花崗岩類中鋯石微量元素組成在岩石成因上的應用

論文名稱(外文):, Trace Element Determination of Zircons from Adakites and Granitoids: Implications for Petrogenetic Processes. 指導教授: 朱美妃;鍾孫霖. 資料載入處理中... 跳到主要內容 臺灣博碩士論文加值系統 ::: 網站導覽| 首頁| 關於本站| 聯絡我們| 國圖首頁| 常見問題| 操作說明 English |FB專頁 |Mobile 免費會員 登入| 註冊 功能切換導覽列 (167.99.71.17)您好！臺灣時間：2022/06/1712:37 字體大小：       ::: 詳目顯示 recordfocus 第1筆/ 共1筆  /1頁 論文基本資料 摘要 外文摘要 目次 參考文獻 紙本論文 QRCode 本論文永久網址: 複製永久網址Twitter研究生:陳采薇研究生(外文):Tsai-WeiChen論文名稱:埃達克岩與花崗岩類中鋯石微量元素組成在岩石成因上的應用論文名稱(外文):TraceElementDeterminationofZirconsfromAdakitesandGranitoids:ImplicationsforPetrogeneticProcesses指導教授:朱美妃、鍾孫霖口試日期:2017-07-24學位類別:碩士校院名稱:國立臺灣大學系所名稱:地質科學研究所學門:自然科學學門學類:地球科學學類論文種類:學術論文論文出版年:2017畢業學年度:105語文別:中文論文頁數:219中文關鍵詞:鋯石、埃達克岩、花崗岩類、微量元素組成、地球化學判別因子外文關鍵詞:zircon、adakites、granitoids、traceelementcomposition、geochemicaldiscriminants相關次數: 被引用:0點閱:165評分:下載:0書目收藏:0 在地球演化相關研究中，鋯石長期以來被視為可以記述大陸地殼演化的時空膠囊。

根據前人的地球化學分析結果知道大陸地殼平均組成在晚太古宙從TTG岩套轉變為花崗岩類，鑑於鋯石對親岩元素有較高的相容性，一般認為其有機會將岩漿的化學成分差異記錄在組成中。

因為埃達克岩為TTG岩套的現代類比，所以本研究針對西藏南部後碰撞埃達克岩、岡底斯I型花崗岩類、蘇門答臘高/低總REE濃度花崗岩類以及多巴火山岩的岩漿鋯石進行電子微探和雷射剝蝕感應耦合電漿質譜原位分析，分別利用這兩個方法測量鋯石中三個主量元素和二十九個微量元素的含量，並比較埃達克岩與花崗岩類的鋯石化學組成。

結果顯示本研究的鋯石組成成分為31.4–34.8wt.%的SiO2、60.2–68.6wt.%的ZrO2、0.6–2.4wt.%的HfO2，以及200–5000ppm的稀土元素，並在稀土元素分配圖上呈現Ce與Eu的異常，而儘管埃達克岩相對花崗岩類的全岩組成具有明顯的重稀土元素虧損現象，但在鋯石稀土元素分配圖上樣本間幾乎不存在區別。

並且任一項鋯石化學組成特徵皆未與全岩SiO2含量和ASI產生相關性，指示結晶分異作用不會對鋯石的組成造成顯著影響。

本研究認為鋯石無法像全岩可以反映埃達克岩及花崗岩類的組成差異，除了晶格應變和電荷平衡要求的影響之外，亦可能起因於樣本中的鋯石是在晶漿環境中生長，周圍的岩漿已經演化到中後期，所以不同群體鋯石所記錄的岩漿組成並非平均熔體成分，且彼此差異很小；另一方面，先於或與鋯石同時結晶的礦物相(如磷灰石、獨居石等)也會降低熔體中輕稀土元素和中稀土元素的含量，所以會將岡底斯埃達克岩鋯石原本應該繼承的重稀土元素虧損特性消除掉。

雖然上述結果顯示埃達克岩與花崗岩類中的鋯石無明顯的化學成分差別，但本研究嘗試利用統計分析對龐大的鋯石微量元素組成資料庫進行處理，目的是為了客觀挑選出埃達克岩和花崗岩類鋯石中其他的成分判別因子，最後共選出Ti、V、Yb、Hf、Sc/Yb、U/Yb、Eu/Eu*、ΣHREE等八個判別因子。

即使統計分析的結果無法利用雙變數圖分開埃達克岩和花崗岩類的鋯石群體，判別因子的線性組合仍可以提供一個有潛力的族群判別方式，將兩個鋯石群體分開。

Zirconhaslongbeenproposedasatimecapsuleofcrustalformation.Concerningofitshighcapacityoflithophileelements,thedramaticchangeincrustalchemicalcompositioninlateArchean,i.e.fromTTGsuitestogranitoids,mayberecordedinzirconremnants.Inthisstudy,geochemicalcontentsofzirconsfromadakites,amodernanalogueofTTGsuites,insouthernTibetweredeterminedandcomparedwiththoseinGangdeseI-typegranitoids,Sumatrahigh/lowΣREEgranitoidsandTobavolcanicsinordertoexaminethehypothesis.Forzirconsineachsamplegroup,electronprobemicroanalysisandlaserablation-inductivelycoupledplasmamassspectrometrywereconductedinordertoprovideinsituconcentrationsof3major-and29traceelements,respectively.Zirconsinthisstudyhaveacommoncompositionof31.4–34.8wt.%SiO2,60.2–68.6wt.%ZrO2,and0.6–2.4wt.%HfO2withΣREEabundancesof200–5000ppm,CepositiveanomalyandEunegativeanomalyinREEpatterns.TheREEpatternsofzirconsshowlittleinter-samplediscrepancythoughthereissignificantdifferenceinwhole-rockHREEcontentsbetweenadakitesandgranitoids.Sincenoneofgeochemicalfeature,includingREEcontents,ofzirconsinthisstudycorrelateswithSiO2contentorASIofcorrespondinghostrocks,fractionalcrystallizationhasaninsignificantimpactonthecompositionalvariationinzircons.Inadditiontotheinfluenceoflatticestrainandchargebalancerequirements,zirconsintheserocksamplesareproposedtocrystallizefromthemagmamush,sotheyrecordthecompositionofevolvedmagmawithleastcompositiondifference,notthatofthebulkmelt.Morespecifically,thepre-/co-existingmineralphases,i.e.apatite,monazite,etc.,playacriticalroleinpreferentiallytakingtheLREEandMREEfrommelt,andeliminatingtheHREEdepletioncharacteristicsinresidualmeltandthuszirconsofGangdeseadakites.Withtheaimofobjectivelyidentifyinggeochemicaldiscriminantsofzirconsfromadakitesandgranitoids,statisticalanalysiswasusedandthen8parameterswereselected,i.e.Ti,V,Yb,Hf,Sc/Yb,U/Yb,Eu/Eu*,ΣHREE.Despitethefactthatthezirconpopulationsofadakites-andgranitoids-originsmoreorlessoverlapinanybivariateplot,thelinearcombinationofdiscriminantsprovidesapotentialwaytodistinguishzirconsfromthesetwogroups. 口試委員審定書I誌謝II中文摘要IVAbstractVI目錄VIII圖目錄X表目錄XIV第一章緒論11.1研究動機11.1.1埃達克岩與花崗岩類11.1.2礦物組成分析31.2研究目的5第二章文獻回顧62.1鋯石微量元素組成62.1.1鋯石結構與組成62.1.2微量元素組成圖解102.2地質背景162.2.1埃達克岩162.2.2花崗岩類182.2.3火山岩21第三章研究方法243.1研究區域與樣本資訊243.2樣本靶製作與影像363.3儀器分析403.3.1能量分散式光譜儀403.3.2電子微探分析儀403.3.3雷射剝蝕感應耦合電漿質譜儀423.4資料處理463.4.1單變量統計分析463.4.2多變量統計分析47第四章研究結果504.1鋯石外型及內部觀察504.2鋯石主量元素分析結果584.3鋯石微量元素分析結果664.4統計分析結果784.4.1單變量統計分析784.4.2多變量統計分析85第五章討論875.1鋯石稀土元素特徵875.1.1鈰與銪異常875.1.2稀土元素分配圖形對比925.2鋯石微量元素組成於岩石成因之應用955.2.1晶漿環境955.2.2共生礦物相競爭975.3埃達克岩及花崗岩類之鋯石組成判別1025.3.1前人鋯石微量元素判別規則1025.3.2判別函數105第六章結論112參考文獻114附錄一、附圖及附表127附錄二、統計分析程式碼218 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